Mechanochemical Ni-Catalysed Arylation of Ortho-Hydroxyarylenaminones: Synthesis of Isoflavones

DC ElementWertSprache
dc.contributor.authorMkrtchyan, Satenik
dc.contributor.authorJakubczyk, Michal
dc.contributor.authorLanka, Suneel
dc.contributor.authorYar, Muhammad
dc.contributor.authorMahmood, Tariq
dc.contributor.authorAyub, Khurshid
dc.contributor.authorSillanpaa, Mika
dc.contributor.authorThomas, Christine M.
dc.contributor.authorIaroshenko, Viktor O.
dc.date.accessioned2023-02-17T11:36:54Z-
dc.date.available2023-02-17T11:36:54Z-
dc.date.issued2022
dc.identifier.issn1615-4150
dc.identifier.urihttp://osnascholar.ub.uni-osnabrueck.de/handle/unios/65636-
dc.description.abstractThis work describes two new synthetic methods for the preparation of isoflavones following the Ni-catalysed domino arylation reactions of the vast range of ortho-hydroxyarylenaminones utilising aromatic bromides as well as carboxylic acids. The presented protocols tolerated significant variation of all coupling partners and enabled synthesis of isoflavone library of twenty-three representatives. This is the first communicated precedent where the mechanic energy was utilised in the synthesis of isoflavones following the domino cyclisation mode.
dc.description.sponsorshipAgentura na podporu vyskumu a vyvoja'' Slovakia [APVV-21-0362]; This research project was supported by a grant (Nr. APVV-21-0362) from ``Agentura na podporu vyskumu a vyvoja'' Slovakia.
dc.language.isoen
dc.publisherWILEY-V C H VERLAG GMBH
dc.relation.ispartofADVANCED SYNTHESIS & CATALYSIS
dc.subjectANALOGS
dc.subjectArylation
dc.subjectARYLBORONIC ACIDS
dc.subjectCASCADES
dc.subjectCatalysis
dc.subjectChemistry
dc.subjectChemistry, Applied
dc.subjectChemistry, Organic
dc.subjectCROSS-COUPLING REACTION
dc.subjectDERIVATIVES
dc.subjectH BOND TRIFLUOROMETHYLATION
dc.subjectIsoflavones
dc.subjectMechanochemistry
dc.subjectMethodology
dc.subjectPROPARGYLIC ALCOHOLS
dc.subjectSTRATEGY
dc.subjectWATER
dc.titleMechanochemical Ni-Catalysed Arylation of Ortho-Hydroxyarylenaminones: Synthesis of Isoflavones
dc.typejournal article
dc.identifier.doi10.1002/adsc.202200645
dc.identifier.isiISI:000842303100001
dc.description.volume364
dc.description.issue20
dc.description.startpage3512
dc.description.endpage3521
dc.contributor.orcid0000-0003-0990-1860
dc.contributor.orcid0000-0002-5647-5326
dc.contributor.orcid0000-0002-6277-5800
dc.contributor.researcheridI-8117-2013
dc.identifier.eissn1615-4169
dc.publisher.placePOSTFACH 101161, 69451 WEINHEIM, GERMANY
dcterms.isPartOf.abbreviationAdv. Synth. Catal.
local.import.remainsaffiliations : Matej Bel University; Polish Academy of Sciences; Lodz University of Technology; COMSATS University Islamabad (CUI); King Saud University; Universiti Kebangsaan Malaysia; Aarhus University; University System of Ohio; Ohio State University; University of Helsinki; University Osnabruck
local.import.remainsearlyaccessdate : AUG 2022
local.import.remainsweb-of-science-index : Science Citation Index Expanded (SCI-EXPANDED); Index Chemicus (IC); Current Chemical Reactions (CCR-EXPANDED)
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